Ultrafast Time-and-Space- Domain Holography by Spectral Hole Burning in Dye-Doped Polymers

Abstract

Certain photochromic materials exhibit at liquid-helium temperature a special property of very high selectivity in frequency dimension. This phenomenon, commonly known as spectral hole burning (SHB), makes it possible to extend conventional spatial-domain optical data storage into the dimensions of frequency and time. We have applied SHB for ultrafast recording of holograms and coherent optical processing on the timescale of 10^-12–10^-13 s. To achieve ultrafast performance in the time domain, we use special organic dye-doped polymer materials, which provide SHB recording in a broad optical band width of 5–10 THz. In this paper, we discuss recording and playback of holograms of pico- and femtosecond time-and-space-domain signals using dye-doped SHB polymers at liquid-helium temperature. We discuss unusual properties of SHB holograms such as causality-related asymmetry of diffraction and inversion of the time coordinate, ultrafast frequency-domain processing, and associative recall of events.